ABSTRACT

A detectable nonlinear response between light and matter depends on one of two key ingredients: Either there is a resonance between the light wave and some natural oscillation mode of the material, or the light is sufficiently intense. In this chapter, the authors let the matter variables themselves play active roles and derive coupled nonlinear differential equations for the electric and matter fields. They outline the use of Schrodinger's equation to derive the Bloch equations, which describe the dynamics of the oscillators of matter and help to derive the Maxwell equation for the envelope of an almost monochromatic electromagnetic wave. The authors analyse the case of two distinct co- or counter-propagating waves interacting with a three-level medium where both waves excite separate quantum transitions sharing a common level. They also help to derive an effective two-level atom model that describes two-photon absorption and stimulated Raman scattering.