ABSTRACT

As we just described above, the hyperfine interaction with randomly ori-

ented nuclear spins is a fundamental decoherence mechanism for electron

spin in a semiconductor quantum dot. However, the nuclear spins them-

selves could be used to create long-lived quantum memory for quantum

bits. Nuclear spins can possess very long coherence times because of their

weak environmental coupling, but single nuclear spins are very difficult to

manipulate and measure [8]. A recent proposal by Taylor et al is moti-

vated by the possibility to use the nuclear spins as a quantum memory and

aims to combine the strengths of electron-spin (or charge) manipulation

with the long-term memory provided by the nuclear spin system [16]. The

target is to achieve a nuclear polarisation degree that is high enough to

transfer a coherent spin state from a single electron to the nuclear spin

system. This is achieved through the effective control of the spin-exchange

part of hyperfine contact interaction (via an external magnetic field pulse

for instance). After the transfer is completed, the resulting superpositions

could be stored for very long times and mapped back into the electron spin

degrees of freedom on demand. It would thus be possible to reliably map

the quantum state of a spin qubit onto long-lived collective nuclear-spin

states. This proposal is quite similar to the use of atomic ensembles as

quantum information carriers [72]. The experimental implementation of

this technique will require on the one hand, a strong strong nuclear-spin

polarization in the vicinity of confined electrons, and on the other hand

long carrier spin life and coherence times, see section 9.4. We have thus

performed a detailed investigation of the nuclear spin polarization in self-

organized InAs/GaAs quantum dots. Achieving a very large nuclear spin

polarization would (i) limit the fundamental decoherence mechanism for

electron spin in a quantum dot [28, 73] (see section 9.4) and (ii) opens the

route towards the implementation of quantum memories based on collective

nuclear spin states.